The assay of Vitamin B1 (thiamine) by fluorimetry involves measuring the fluorescence emitted by thiamine or its derivatives after a specific chemical reaction that enhances its fluorescence. Here's an overview of the steps involved in this assay:
1. Principle:
Vitamin B1 (thiamine) itself is not strongly fluorescent. However, when it is oxidized to thiochrome, a highly fluorescent compound, the fluorescence can be measured using a fluorimeter. The intensity of the fluorescence is directly proportional to the concentration of thiamine in the sample.
2. Preparation of Sample:
- Extraction: Thiamine is extracted from the sample (biological fluids, food, etc.) by hydrolysis under acidic conditions.
- Neutralization: After extraction, the sample is neutralized to prevent further degradation of thiamine.
3. Oxidation to Thiochrome:
- Oxidation Reaction: Thiamine is treated with an oxidizing agent, typically alkaline potassium ferricyanide. This converts thiamine into its fluorescent derivative, thiochrome.
- The reaction occurs in alkaline conditions (pH around 12-13).
4. Fluorescence Measurement:
- The fluorescence of thiochrome is measured using a fluorimeter.
- Excitation wavelength: Thiochrome is excited at around 365 nm.
- Emission wavelength: The emitted fluorescence is measured at around 435-440 nm.
5. Quantification:
- A calibration curve is generated using known concentrations of thiamine standards.
- The fluorescence intensity of the sample is compared to the calibration curve to determine the concentration of Vitamin B1 in the sample.
6. Advantages of Fluorimetry:
- Sensitivity: Fluorimetry is highly sensitive, making it suitable for detecting low concentrations of Vitamin B1.
- Specificity: The assay is relatively specific to Vitamin B1, provided the extraction and oxidation steps are performed carefully.
7. Limitations:
- The method requires careful handling during oxidation to avoid over-oxidation or degradation of thiamine.
- Fluorescence measurements are sensitive to environmental factors like light and temperature, so proper control measures are necessary.
In conclusion, fluorimetry provides a sensitive and reliable method to assay Vitamin B1 by converting it into its fluorescent form, thiochrome, and measuring the fluorescence intensity.
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